Additional global climate cooling by clouds due to ice crystal complexity

TitleAdditional global climate cooling by clouds due to ice crystal complexity
Publication TypeJournal Article
Year of Publication2018
AuthorsJarvinen E., Jourdan O., Neubauer D., Yao B., Liu C., Andreae M.O, Lohmann U., Wendisch M., McFarquhar G.M, Leisner T., Schnaiter M.
JournalAtmospheric Chemistry and Physics
Volume18
Pagination15767-15781
Date Published2018/11
Type of ArticleArticle
ISBN Number1680-7316
Accession NumberWOS:000449342400003
Keywordsairborne polar nephelometer; cirrus clouds; in-situ; measurements; Meteorology & Atmospheric Sciences; microphysical properties; observations; particle habit; polarization; radiance measurements; radiative properties; single-scattering properties; surface-roughness
Abstract

Ice crystal submicron structures have a large impact on the optical properties of cirrus clouds and consequently on their radiative effect. Although there is growing evidence that atmospheric ice crystals are rarely pristine, direct in situ observations of the degree of ice crystal complexity are largely missing. Here we show a comprehensive in situ data set of ice crystal complexity coupled with measurements of the cloud angular scattering functions collected during a number of observational airborne campaigns at diverse geographical locations. Our results demonstrate that an overwhelming fraction (between 61% and 81%) of atmospheric ice crystals sampled in the different regions contain mesoscopic deformations and, as a consequence, a similar flat and featureless angular scattering function is observed. A comparison between the measurements and a database of optical particle properties showed that severely roughened hexagonal aggregates optimally represent the measurements in the observed angular range. Based on this optical model, a new parameterization of the cloud bulk asymmetry factor was introduced and its effects were tested in a global climate model. The modelling results suggest that, due to ice crystal complexity, ice-containing clouds can induce an additional short-wave cooling effect of -1.12 W m(2) on the top-of-the-atmosphere radiative budget that has not yet been considered.

DOI10.5194/acp-18-15767-2018
Short TitleAtmos. Chem. Phys.
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