African volcanic emissions influencing atmospheric aerosols over the Amazon rain forest

TitleAfrican volcanic emissions influencing atmospheric aerosols over the Amazon rain forest
Publication TypeJournal Article
Year of Publication2018
AuthorsSaturno J., Ditas F., de Vries M.P, Holanda B.A, Pohlker M.L, Carbone S., Walter D., Bobrowski N., Brito J., Chi X.G, Gutmann A., de Angelis I.H, Machado L.AT, Moran-Zuloaga D., Rudiger J., Schneider J., Schulz C., Wang Q.Q, Wendisch M., Artaxo P., Wagner T., Poschl U., Andreae M.O, Pohlker C.
JournalAtmospheric Chemistry and Physics
Volume18
Pagination10391-10405
Date Published2018/07
Type of ArticleArticle
ISBN Number1680-7316
Accession NumberWOS:000439427800001
Keywordsbasin; dry season; lava lake; light-absorption; long-term; Meteorology & Atmospheric Sciences; ozone monitoring instrument; part 1; satellite-observations; so2; wet season
Abstract

The long-range transport (LRT) of trace gases and aerosol particles plays an important role for the composition of the Amazonian rain forest atmosphere. Sulfate aerosols originate to a substantial extent from LRT sources and play an important role in the Amazonian atmosphere as strongly light-scattering particles and effective cloud condensation nuclei. The transatlantic transport of volcanic sulfur emissions from Africa has been considered as a source of particulate sulfate in the Amazon; however, direct observations have been lacking so far. This study provides observational evidence for the influence of emissions from the Nyamuragira-Nyiragongo volcanoes in Africa on Amazonian aerosol properties and atmospheric composition during September 2014. Comprehensive ground-based and airborne aerosol measurements together with satellite observations are used to investigate the volcanic event. Under the volcanic influence, hourly mean sulfate mass concentrations in the submicron size range reached up to 3.6 mu gm(3) at the Amazon Tall Tower Observatory, the highest value ever reported in the Amazon region. The substantial sulfate injection increased the aerosol hygroscopicity with kappa values up to 0.36, thus altering aerosol-cloud interactions over the rain forest. Airborne measurements and satellite data indicate that the transatlantic transport of volcanogenic aerosols occurred in two major volcanic plumes with a sulfate-enhanced layer between 4 and 5 km of altitude. This study demonstrates how African aerosol sources, such as volcanic sulfur emissions, can substantially affect the aerosol cycling and atmospheric processes in Amazonia.

DOI10.5194/acp-18-10391-2018
Short TitleAtmos. Chem. Phys.
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